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Photocatalytic sacrificial H2 evolution dominated by micropore-confined exciton transfer in hydrogen-bonded organic frameworks - Nature Catalysis

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Photocatalytic sacrificial H2 evolution dominated by micropore-confined exciton transfer in hydrogen-bonded organic frameworks - Nature Catalysis

Organic semiconductors are attractive photocatalysts, but their quantum yields are limited by the transfer of photogenerated charges to the surface. A promising strategy for low-loss charge transfer is to shorten the distance from the bulk exciton coupling region to the catalyst surface. Here we employ the hydrogen-bonded organic framework 1,3,6,8-tetrakis(p-benzoic acid)pyrene (HOF-H4TBAPy) with hydrophilic one-dimensional micropore channels as a proof of concept for this approach.

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Photocatalytic sacrificial H2 evolution dominated by micropore-confined exciton transfer in hydrogen-bonded organic frameworks - Nature Catalysis

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Photocatalytic sacrificial H2 evolution dominated by micropore-confined exciton transfer in hydrogen-bonded organic frameworks - Nature Catalysis

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