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Nanoconfined polymerization limits crack propagation in hysteresis-free gels - Nature Materials

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Nanoconfined polymerization limits crack propagation in hysteresis-free gels - Nature Materials

Consecutive mechanical loading cycles cause irreversible fatigue damage and residual strain in gels, affecting their service life and application scope. Hysteresis-free hydrogels within a limited deformation range have been created by various strategies. However, large deformation and high elasticity are inherently contradictory attributes. Here we present a nanoconfined polymerization strategy for producing tough and near-zero-hysteresis gels under a large range of deformations.

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Nanoconfined polymerization limits crack propagation in hysteresis-free gels - Nature Materials

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Nanoconfined polymerization limits crack propagation in hysteresis-free gels - Nature Materials

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