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Rotation in attosecond vibronic coherence spectroscopy for molecules - Communications Physics

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Rotation in attosecond vibronic coherence spectroscopy for molecules - Communications Physics

Excitation or ionization of a molecule by ultrafast laser pulses can create a superposition of electronic states, whose dynamics is influenced by the interplay of electronic coherence and nuclear motion, resulting in charge migration and possibly charge transfer. Probing the vibronic coherence is therefore vital to monitoring electronic dynamics and controlling chemical reactivity, as recently demonstrated in molecules via attosecond transient absorption spectroscopy (ATAS).

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Rotation in attosecond vibronic coherence spectroscopy for molecules - Communications Physics

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